X-ray free-electron lasers (FELs), which amplify light emitted by a relativistic electron beam, are extending nonlinear optical tech- niques to shorter wavelengths, adding element specificity by exciting and probing electronic transitions from core levels. These techniques would benefit tremendously from having a stable FEL source, generating spectrally pure and wavelength-tunable pulses. We show that such requirements can be met by operating the FEL in the so-called echo-enabled harmonic generation (EEHG) con- figuration. Here, two external conventional lasers are used to precisely tailor the longitudinal phase space of the electron beam before emission of X-rays. We demonstrate high-gain EEHG lasing producing stable, intense, nearly fully coherent pulses at wave- lengths as short as 5.9 nm (~211 eV) at the FERMI FEL user facility. Low sensitivity to electron-beam imperfections and observa- tion of stable, narrow-band, coherent emission down to 2.6 nm (~474 eV) make the technique a prime candidate for generating laser-like pulses in the X-ray spectral region, opening the door to multidimensional coherent spectroscopies at short wavelengths.

Coherent soft X-ray pulses from an echo-enabled harmonic generation free-electron laser / Rebernik Ribic, P., Abrami, A., Badano, L., Bossi, M., Braun, H.-H., Bruchon, N., Capotondi, F., Castronovo, D., Cautero, M., Cinquegrana, P., Coreno, M., Couprie, M.E., Cudin, I., Boyanov Danailov, M., De Ninno, G., Demidovich, A., Di Mitri, S., Diviacco, B., Fawley, W.M., Feng, C., et al.. - In: NATURE PHOTONICS. - ISSN 1749-4885. - 13:8(2019), pp. 555-561. [10.1038/s41566-019-0427-1]

Coherent soft X-ray pulses from an echo-enabled harmonic generation free-electron laser

Bruchon N.;Capotondi F.;De Ninno G.;Ferrari E.;Grattoni V.;Malvestuto M.;Veronese M.;
2019-01-01

Abstract

X-ray free-electron lasers (FELs), which amplify light emitted by a relativistic electron beam, are extending nonlinear optical tech- niques to shorter wavelengths, adding element specificity by exciting and probing electronic transitions from core levels. These techniques would benefit tremendously from having a stable FEL source, generating spectrally pure and wavelength-tunable pulses. We show that such requirements can be met by operating the FEL in the so-called echo-enabled harmonic generation (EEHG) con- figuration. Here, two external conventional lasers are used to precisely tailor the longitudinal phase space of the electron beam before emission of X-rays. We demonstrate high-gain EEHG lasing producing stable, intense, nearly fully coherent pulses at wave- lengths as short as 5.9 nm (~211 eV) at the FERMI FEL user facility. Low sensitivity to electron-beam imperfections and observa- tion of stable, narrow-band, coherent emission down to 2.6 nm (~474 eV) make the technique a prime candidate for generating laser-like pulses in the X-ray spectral region, opening the door to multidimensional coherent spectroscopies at short wavelengths.
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11368/2948506
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